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81.
Yanan Xu Kai Wang Jianwei Han Cong Liu Yabin An Qinghai Meng Chen Li Xiong Zhang Xianzhong Sun Yaosheng Zhang Lijuan Mao Zhixiang Wei Yanwei Ma 《Advanced materials (Deerfield Beach, Fla.)》2020,32(45):2005531
Smart and wearable electronics have aroused substantial demand for flexible portable power sources, but it remains a large challenge to realize scalable production of wearable batteries/supercapacitors with high electrochemical performance and remarkable flexibility simultaneously. Here, a scalable approach is developed to prepare wearable solid-state lithium-ion capacitors (LICs) with superior performance enabled by synergetic engineering from materials to device architecture. Nitrogen-doped hierarchical carbon (HC) composed of 1D carbon nanofibers welded with 2D carbon nanosheets is synthesized via a unique self-propagating high-temperature synthesis (SHS) technique, which exhibits superior electrochemical performance. Subsequently, inspired by origami, here, wave-shaped LIC punch-cells based on the above materials are designed by employing a compatible and scalable post-imprint technology. Finite elemental analysis (FEA) confirms that the bending stress of the punch-cell can be offset effectively, benefiting from the wave architecture. The wearable solid-state LIC punch-cell exhibits large energy density, long cyclic stability, and superior flexibility. This study demonstrates great promise for scalable fabrication of wearable energy-storage systems. 相似文献
82.
83.
分析反应堆压力容器(RPV)锻件制造过程中关键化学元素含量及基准无塑性转变温度(RTNDT)数值,通过引入修正淬透性系数,建立了反映RTNDT变化规律的修正淬透性系数函数表达式,并给出了实例验证,结果表明,通过本文建立的修正淬透性系数函数式可以比较精确地预估RPV锻件的RTNDT值。 相似文献
84.
苯并噁嗪树脂作为一类新型的热固性树脂,具有分子设计性强、阻燃性能和耐腐蚀性能优异、固化时不需要强酸、无小分子放出等优点,在航空、建筑、电子等领域获得了广泛应用。本文主要介绍了苯并噁嗪单体的合成方法(溶剂法、无溶剂法和悬浮法)、降低苯并噁嗪开环聚合温度的方法(合成具有特殊基团的苯并噁嗪单体、添加催化剂)及苯并噁嗪树脂在形状记忆聚合物中的应用(与其他聚合物混合,纯苯并噁嗪化学改性),对苯并噁嗪形状记忆聚合物目前存在的问题进行了概述并对苯并噁嗪形状记忆聚合物的发展前景做出了展望。 相似文献
85.
Wireless Networks - In such mobile platforms as ships and aircraft, the detection and reconnaissance devices are near to the communication facilities. When working at the same time, they will... 相似文献
86.
Bing Huang Meng Wang Guodong Xu Lin Hu Lin Chen Yijie Gu 《Ceramics International》2021,47(6):7700-7710
In this study, La was doped into the lithium layer of Li-rich cathode material and formed a layered-spinel hetero-structure. The morphology, crystal structure, element valence and kinetics of lithium ion migration were studied by field emission scanning electron microscope (FESEM), X-ray diffraction (XRD), X-ray photoelectron spectroscopy (XPS) and electrochemical impedance spectroscopy (EIS). The La doped lithium-rich cathode material exhibited similar initial discharge capacity of 262.8 mAh g?1 at 0.1 C compared with the undoped material, but the discharge capacity retention rate can be obviously improved to 90% after 50 cycles at 1.0 C. Besides that, much better rate capability and Li+ diffusion coefficient were observed. The results revealed that La doping not only stabilized the material structure and reduced the Li/Ni mixing degree, but also induced the generation of spinel phase to provide three-dimensional diffusion channels for lithium ion migration. Moreover, the porous structure of the doped samples also contributed to the remarkable excellent electrochemical performance. All of these factors combined to significantly improve the electrochemical performance of the material. 相似文献
88.
Runze Mao Jinhua Wang Weijie Zhang Zhenhua An Wenjun Lin Meng Zhang Zuohua Huang 《International Journal of Hydrogen Energy》2021,46(34):17969-17981
In this study, we investigated the H2-induced transition of confined swirl flames from the “V” to “M” shape. H2-enriched lean premixed CH4/H2/air flames with H2 fractions up to 80% were conducted. The flame structure was obtained with Planar Laser-Induced Fluorescence (PLIF) of the OH radical. Flow fields were measured with Particle Image Velocimetry (PIV). It was observed that the flame tip in the outer shear layer gradually propagated upstream and finally anchored to the injector with the hydrogen fractions increase, yielding the transition from the “V” to “M” flame. We examined the flame structures and the flame flow dynamics during the transition. The shape transition was directly related to the evolution of the corner flame along the outer shear layer. With H2 addition, the outer recirculation zone first appeared downstream where the corner flame started to propagate upstream; then, the recirculation zone expanded upward to form a stable “M” flame gradually. The flow straining was observed to influence the stabilization of the outer shear layer flame significantly. This study can be useful for the understanding of recirculation-stabilized swirling flames with strong confinement. The flame structure and the flow characteristics of flames with a high H2 content are also valuable for model validation. 相似文献
89.
Senliang Xi Xiaojun Wang Kudzaishe Caren Tome Tonghuan Zhang Zongying Han Meng Gao Shixue Zhou Hao Yu 《International Journal of Hydrogen Energy》2021,46(46):23748-23756
The hydrogen storage performances of MgH2 improved by the addition of Ni and SAPO-34 were studied in detail. The mixture of MgH2 with Ni and SAPO-34 was a physical reaction as shown by the X-ray diffraction (XRD) results. The SAPO-34 and Ni were uniformly distributed on the surface of MgH2. The thermodynamic and kinetic properties of 90MgH2/5Ni/5SAPO-34 were investigated by differential scanning calorimetry (DSC) and pressure-composition-isothermal (PCI) methods. The results showed that the dehydrogenation activation energy of 90MgH2/5Ni/5SAPO-34 decreased by 64.3 kJ/mol compared with that of MgH2. In addition, the relationship between the value of dehydrogenation heat and hydrogen content was also investigated by in-situ calorimetry. The enthalpy value of each sample in the dehydrogenation processes were calculated by in-situ calorimetry measurement. The dehydrogenation enthalpies of as-milled MgH2 and 90MgH2/5Ni/5SAPO-34 were 63.2 kJ/mol H2 and 53.6 kJ/mol H2, respectively. Thus, the co-doping of Ni and SAPO-34 contributed significantly to decrease the thermodynamic stability and improve the hydrogen sorption kinetic properties of MgH2. 相似文献
90.